Residential College | false |
Status | 已發表Published |
Multi-Component Crosslinked Hydrogel Electrolyte toward Dendrite-Free Aqueous Zn Ion Batteries with High Temperature Adaptability | |
Lu, Hongyu1,2; Hu, Jisong3; Wang, Litong4; Li, Jianzhu1,2; Ma, Xiang2; Zhu, Zhicheng2; Li, Heqi2; Zhao, Yingjie2; Li, Yujie1,2; Zhao, Jingxin5; Xu, Bingang5 | |
2022-01-27 | |
Source Publication | Advanced Functional Materials |
ISSN | 1616-301X |
Volume | 32Issue:19Pages:2112540 |
Abstract | Rechargeable aqueous Zn-ion batteries (ZIBs) are always regarded as a promising energy storage device owing to their higher safety and durability. However, two problems have become the main trouble for the practical application of ZIBs such as the dendrite growth of Zn metal anode in electrolyte and the freezing of water solvent at low temperature. Herein, to overcome these challenges, a new strategy, multi-component crosslinked hydrogel electrolyte, is proposed to inhibit Zn dendrites and realize low temperature environmental adaptability for ZIBs. Benefitting from the superior inhibition effect of the polyacrylamide and dimethyl sulfoxide (DMSO) on Zn dendrites, the coulombic efficiency of the symmetric cell of ≈99.5% is achieved during the Zn plating/stripping over 1 300 h, and the assembled full-cell demonstrates the large specific capacity of 265.2 mAh g-1 and high cyclic stability with the capacity retention of 95.27% after 3 000 cycles. In addition, the full-cell delivers stable operation at a wide temperature range, from 60 to −40 °C, due to the introduction of additive DMSO. This work provides an inspired strategy and novel opportunities to realize a dendrite-free and wide-temperature rechargeable aqueous Zn-ion energy storage system. |
Keyword | Aqueous Zn Ion Batteries Highly Reversible Zn Anodes Hydrogel Electrolytes Wide-temperature Range Zn Dendrites |
DOI | 10.1002/adfm.202112540 |
URL | View the original |
Indexed By | SCIE |
Language | 英語English |
WOS Research Area | Chemistry ; Science & Technology - Other Topics ; Materials Science ; Physics |
WOS Subject | Chemistry, Multidisciplinary ; Chemistry, Physical ; Nanoscience & Nanotechnology ; Materials Science, Multidisciplinary ; Physics, Applied ; Physics, Condensed Matter |
WOS ID | WOS:000747600900001 |
Publisher | WILEY-V C H VERLAG GMBH |
Scopus ID | 2-s2.0-85123789472 |
Fulltext Access | |
Citation statistics | |
Document Type | Journal article |
Collection | INSTITUTE OF APPLIED PHYSICS AND MATERIALS ENGINEERING |
Corresponding Author | Li, Yujie; Zhao, Jingxin; Xu, Bingang |
Affiliation | 1.State Key Laboratory of Advanced Welding and Joining, Harbin Institute of Technology, Harbin, 150001, China 2.School of Materials Science and Engineering, Harbin Institute of Technology (Weihai), Weihai, 264209, China 3.School of Optical and Electronic Information, Huazhong University of Science and Technology, Wuhan, 430074, China 4.Joint Key Laboratory of the Ministry of Education, Institute of Applied Physics and Materials Engineering, University of Macau, Avenida da Universidade, Taipa, SAR, 999078, Macao 5.Nanotechnology Center, Institute of Textiles and Clothing, The Hong Kong Polytechnic University, Kowloon, Hung Hom, 999077, Hong Kong |
Recommended Citation GB/T 7714 | Lu, Hongyu,Hu, Jisong,Wang, Litong,et al. Multi-Component Crosslinked Hydrogel Electrolyte toward Dendrite-Free Aqueous Zn Ion Batteries with High Temperature Adaptability[J]. Advanced Functional Materials, 2022, 32(19), 2112540. |
APA | Lu, Hongyu., Hu, Jisong., Wang, Litong., Li, Jianzhu., Ma, Xiang., Zhu, Zhicheng., Li, Heqi., Zhao, Yingjie., Li, Yujie., Zhao, Jingxin., & Xu, Bingang (2022). Multi-Component Crosslinked Hydrogel Electrolyte toward Dendrite-Free Aqueous Zn Ion Batteries with High Temperature Adaptability. Advanced Functional Materials, 32(19), 2112540. |
MLA | Lu, Hongyu,et al."Multi-Component Crosslinked Hydrogel Electrolyte toward Dendrite-Free Aqueous Zn Ion Batteries with High Temperature Adaptability".Advanced Functional Materials 32.19(2022):2112540. |
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