Residential College | false |
Status | 已發表Published |
Realization of integrative hierarchy by in-situ solidification of ‘semi-cured’ microcilia array in candle flame for robust and flexible superhydrophobicity | |
Chen, Ge1; Dai, Ziyi1; Ding, Sen1; Lei, Ming1; Lin, Jing2; Wang, Shuangpeng1,3; Zhou, Yinning1; Pan, Hui1,3; Zhou, Bingpu1,3 | |
2022-03-15 | |
Source Publication | Chemical Engineering Journal |
ISSN | 1385-8947 |
Volume | 432Pages:134400 |
Abstract | Flexible superhydrophobic surfaces have recently attracted extensive interest owing to the potential for diverse curvatures and emerging flexible electronics. However, the simultaneous realization of mechanical robustness, chemical resistance, and maintained superhydrophobicity during deformation is still challenging. Herein, we introduced an environmental-friendly method to produce the integrative multi-level structures by generating the micro-cilia array in a ‘template-free’ manner, followed with in-situ thermal curing in the candle flame before the complete solidification of the micro-structured surface. Instead of weak physical adhesion (van der Waals forces), the candle soot nanoparticles penetrated into the ‘semi-cured’ micro-cilia surface, along with the high temperature to rapidly cure and generate the PDMS-connected integrative architectures, which effectively avoid the interface between the micro/nano-scaled components to eliminate the mechanical fragility. Comparative investigations confirm that the elevated robustness is attributed by the synergistic effect from the ‘semi-cured’ surface and the formation mechanism of subsequent hierarchical structures. The flexible film thus exhibits significantly improved stability against mechanical damage (ultrasonic processing, adhesive pressing, and linear abrasion), chemical corrosion, and water-jet impalement (∼10.4 m s at ∼ 0.17 MPa). With the realization of co-existent features and real-life applications, the green methodology should be promising to open up an avenue that moves superhydrophobicity further to our world. |
Keyword | Candle Soot Flexibility Microcilia Robust Hierarchy Superhydrophobicity |
DOI | 10.1016/j.cej.2021.134400 |
URL | View the original |
Indexed By | SCIE |
Language | 英語English |
WOS Research Area | Engineering |
WOS Subject | Engineering, Environmental ; Engineering, Chemical |
WOS ID | WOS:000784266700002 |
Publisher | ELSEVIER SCIENCE SAPO BOX 564, 1001 LAUSANNE, SWITZERLAND |
Scopus ID | 2-s2.0-85122257130 |
Fulltext Access | |
Citation statistics | |
Document Type | Journal article |
Collection | INSTITUTE OF APPLIED PHYSICS AND MATERIALS ENGINEERING |
Corresponding Author | Zhou, Bingpu |
Affiliation | 1.Joint Key Laboratory of the Ministry of Education, Institute of Applied Physics and Materials Engineering, University of Macau, Taipa, Avenida da Universidade, 999078, China 2.School of Chemistry and Chemical Engineering, Guangzhou University, Guangzhou, 510006, China 3.Department of Physics and Chemistry, Faculty of Science and Technology, University of Macau, Taipa, Avenida da Universidade, 999078, China |
First Author Affilication | INSTITUTE OF APPLIED PHYSICS AND MATERIALS ENGINEERING |
Corresponding Author Affilication | INSTITUTE OF APPLIED PHYSICS AND MATERIALS ENGINEERING; Faculty of Science and Technology |
Recommended Citation GB/T 7714 | Chen, Ge,Dai, Ziyi,Ding, Sen,et al. Realization of integrative hierarchy by in-situ solidification of ‘semi-cured’ microcilia array in candle flame for robust and flexible superhydrophobicity[J]. Chemical Engineering Journal, 2022, 432, 134400. |
APA | Chen, Ge., Dai, Ziyi., Ding, Sen., Lei, Ming., Lin, Jing., Wang, Shuangpeng., Zhou, Yinning., Pan, Hui., & Zhou, Bingpu (2022). Realization of integrative hierarchy by in-situ solidification of ‘semi-cured’ microcilia array in candle flame for robust and flexible superhydrophobicity. Chemical Engineering Journal, 432, 134400. |
MLA | Chen, Ge,et al."Realization of integrative hierarchy by in-situ solidification of ‘semi-cured’ microcilia array in candle flame for robust and flexible superhydrophobicity".Chemical Engineering Journal 432(2022):134400. |
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