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Lead oxide enables lead volatilization pollution inhibition and phase purity modulation in perovskite quantum dots embedded borosilicate glass
Yang, Bobo1,2; Mei, Shiliang3; He, Haiyang4; Zhu, Yuxuan2; Hu, Rongrong2; Zou, Jun2; Xing, Guichuan3; Guo, Ruiqian1,4,5,6
2022-01
Source PublicationJournal of the European Ceramic Society
ISSN0955-2219
Volume42Issue:1Pages:258-265
Abstract

Embedding all-inorganic cesium lead halide CsPbX (X=Cl, Br, I) perovskite quantum dots (PQDs) PQDs into glass is one of the most effective strategies to improve their optical, thermal and chemical stabilities. Herein, by using PbO instead of PbBr as the lead source, it is effective to lower the melting temperature and reduce the volatilization pollution from lead halide raw materials. Thus, a high-purity CsPbBr PQDs embedded glass with 71.5 % PLQY was successfully prepared. The thermal stability, and photo-aging properties were also improved. By simply changing the halogen element, the red and blue CsPbX PQDs embedded glasses were successfully prepared. The white LED fabricated by coating obtained green/red CsPbX PQDs embedded glass on a blue chip displays high color gamut of 121.9 % NTSC standard and >91.1 % Rec. 2020 standard, which embodies the great potential of PQDs embedded glass in lighting and display fields.

KeywordPerovskite Quantum Dots Borosilicate Glass Phase Purity Light-emitting Diode Display
DOI10.1016/j.jeurceramsoc.2021.09.052
URLView the original
Indexed BySCIE
Language英語English
WOS Research AreaMaterials Science
WOS SubjectMaterials Science, Ceramics
WOS IDWOS:000711318900008
Scopus ID2-s2.0-85116042246
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Citation statistics
Document TypeJournal article
CollectionINSTITUTE OF APPLIED PHYSICS AND MATERIALS ENGINEERING
Corresponding AuthorZou, Jun; Xing, Guichuan; Guo, Ruiqian
Affiliation1.Institute of Future Lighting, Academy for Engineering and Technology, Fudan University, Shanghai, 200433, China
2.School of Science, Shanghai Institute of Technology, Shanghai, 201418, China
3.Institute of Applied Physics and Materials Engineering, University of Macau, Avenida Da Universidade, Taipa, 999078, China
4.Institute for Electric Light Sources, School of Information Science and Technology, Fudan University, Shanghai, 200433, China
5.Zhongshan - Fudan Joint Innovation Center, Zhongshan, 528437, China
6.Yiwu Research Institute of Fudan University, Yiwu, Chengbei Road, 322000, China
Corresponding Author AffilicationINSTITUTE OF APPLIED PHYSICS AND MATERIALS ENGINEERING
Recommended Citation
GB/T 7714
Yang, Bobo,Mei, Shiliang,He, Haiyang,et al. Lead oxide enables lead volatilization pollution inhibition and phase purity modulation in perovskite quantum dots embedded borosilicate glass[J]. Journal of the European Ceramic Society, 2022, 42(1), 258-265.
APA Yang, Bobo., Mei, Shiliang., He, Haiyang., Zhu, Yuxuan., Hu, Rongrong., Zou, Jun., Xing, Guichuan., & Guo, Ruiqian (2022). Lead oxide enables lead volatilization pollution inhibition and phase purity modulation in perovskite quantum dots embedded borosilicate glass. Journal of the European Ceramic Society, 42(1), 258-265.
MLA Yang, Bobo,et al."Lead oxide enables lead volatilization pollution inhibition and phase purity modulation in perovskite quantum dots embedded borosilicate glass".Journal of the European Ceramic Society 42.1(2022):258-265.
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