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Theoretical analysis of thermal boundary conductance of MoS2-SiO2 and WS2-SiO2 interface
Ong, Zhun Yong1; Cai, Yongqing2; Zhang, Gang1; Zhang, Yong Wei1
2021-03-26
Source PublicationNanotechnology
ISSN0957-4484
Volume32Issue:13Pages:135402
Abstract

Understanding the physical processes involved in interfacial heat transfer is critical for the interpretation of thermometric measurements and the optimization of heat dissipation in nanoelectronic devices that are based on transition metal dichalcogenide (TMD) semiconductors. We model the phononic and electronic contributions to the thermal boundary conductance (TBC) variability for the MoS-SiO and WS-SiO interface. A phenomenological theory to model diffuse phonon transport at disordered interfaces is introduced and yields G = 13.5 and 12.4 MW K m at 300 K for the MoS-SiO and WS-SiO interface, respectively. We compare its predictions to those of the coherent phonon model and find that the former fits the MoS-SiO data from experiments and simulations significantly better. Our analysis suggests that heat dissipation at the TMD-SiO interface is dominated by phonons scattered diffusely by the rough interface although the electronic TBC contribution can be significant even at low electron densities (n < 10 cm) and may explain some of the variation in the experimental TBC data from the literature. The physical insights from our study can be useful for the development of thermally aware designs in TMD-based nanoelectronics.

Keyword2d Materials Phonon Thermal Boundary Conductance Transition Metal Dichalcogenides
DOI10.1088/1361-6528/abd208
URLView the original
Indexed BySCIE
Language英語English
WOS Research AreaScience & Technology - Other Topics ; Materials Science ; Physics
WOS SubjectNanoscience & Nanotechnology ; Materials Science, Multidisciplinary ; Physics, Applied
WOS IDWOS:000605468700001
Scopus ID2-s2.0-85099219280
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Citation statistics
Document TypeJournal article
CollectionINSTITUTE OF APPLIED PHYSICS AND MATERIALS ENGINEERING
Corresponding AuthorOng, Zhun Yong
Affiliation1.Institute of High Performance Computing, A*STAR, Singapore, 138632, Singapore
2.Joint Key Laboratory of the Ministry of Education, Institute of Applied Physics and Materials Engineering, University of Macau, Taipa, Macao
Recommended Citation
GB/T 7714
Ong, Zhun Yong,Cai, Yongqing,Zhang, Gang,et al. Theoretical analysis of thermal boundary conductance of MoS2-SiO2 and WS2-SiO2 interface[J]. Nanotechnology, 2021, 32(13), 135402.
APA Ong, Zhun Yong., Cai, Yongqing., Zhang, Gang., & Zhang, Yong Wei (2021). Theoretical analysis of thermal boundary conductance of MoS2-SiO2 and WS2-SiO2 interface. Nanotechnology, 32(13), 135402.
MLA Ong, Zhun Yong,et al."Theoretical analysis of thermal boundary conductance of MoS2-SiO2 and WS2-SiO2 interface".Nanotechnology 32.13(2021):135402.
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