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Limitations and solutions for achieving high-performance perovskite tandem photovoltaics
Yulan Huang1,2; Tanghao Liu2; Dongyang Li1; Dandan Zhao2; Abbas Amini3; Chun Cheng1,4,5; Guichuan Xing2
Source PublicationNano Energy
ISSN2211-2855
2021-10
Abstract

The large light absorption coefficient, long carrier diffusion length, and high defect tolerance enable organic- inorganic lead halide perovskites for excellent photovoltaic performance. The highest certified power conver-sion efficiency of single-junction perovskite solar cells (PSCs) has reported 25.5%. Besides, the bandgap of pe-rovskites can  be  tuned by  engineering their composition. These merits have made perovskites promising candidates for tandem photovoltaics, which can cross over the Shockley-Queisser limit of single-junction PSCs with economic costs. However, there are yet some hurdles in the wide-bandgap and narrow-bandgap subcells as well as interconnected layers (ICLs), which limit the commercial applications of perovskite tandem solar cells (PTSCs). In  this review, we  summarize the  major scientific and technical limitations of  PTSCs. We  firstly demonstrate the configurations and working principles of PTSCs. Then, the developments of front subcells and rear subcells are discussed. Their main drawbacks, implemented technologies, and underlying mechanisms are analyzed in detail. Subsequently, the progress of ICLs which are responsible for guaranteeing continuous current in 2 T PTSCs are discussed. In addition, the stability of PTSCs is also summarized. The purpose of this review is to map and thrive the future development of PTSCs. 

KeywordWide-bandgap Perovskites Narrow-bandgap Solar Cells Interconnected Layers Perovskite Tandem Solar Cells Passivation Contact
Language英語English
DOI10.1016/j.nanoen.2021.106219
URLView the original
Volume88
Pages106219
WOS IDWOS:000703935100002
WOS SubjectChemistry, Physical ; Nanoscience & Nanotechnology ; Materials Science, Multidisciplinary ; Physics, Applied
WOS Research AreaChemistry ; Science & Technology - Other Topics ; Materials Science ; Physics
Indexed BySCIE
Scopus ID2-s2.0-85108075169
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Document TypeReview article
CollectionINSTITUTE OF APPLIED PHYSICS AND MATERIALS ENGINEERING
Corresponding AuthorChun Cheng; Guichuan Xing
Affiliation1.Department of Materials Science and Engineering, Southern University of Science and Technology, Shenzhen, 518055, China
2.Joint Key Laboratory of the Ministry of Education, Institute of Applied Physics and Materials Engineering, University of Macau, Avenida da Universidade, Taipa, Macau, 999078, China
3.Center for Infrastructure Engineering, Western Sydney University, Kingswood, 2751, Australia
4.Key Laboratory of Energy Conversion and Storage Technologies (Southern University of Science and Technology) Ministry of Education, Shenzhen, 518055, China
5.Shenzhen Engineering Research and Development Center for Flexible Solar Cells, Southern University of Science and Technology, Shenzhen, 518055, China
First Author AffilicationINSTITUTE OF APPLIED PHYSICS AND MATERIALS ENGINEERING
Corresponding Author AffilicationINSTITUTE OF APPLIED PHYSICS AND MATERIALS ENGINEERING
Recommended Citation
GB/T 7714
Yulan Huang,Tanghao Liu,Dongyang Li,et al. Limitations and solutions for achieving high-performance perovskite tandem photovoltaics[J]. Nano Energy, 2021, 88, 106219.
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