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One-Step Inkjet Printed Perovskite in Air for Efficient Light Harvesting
Liang,Chao1; Li,Pengwei1; Gu,Hao1; Zhang,Yiqiang1; Li,Fengyu4; Song,Yanlin4; Shao,Guosheng1; Mathews,Nripan3; Xing,Guichuan2
2018-02-01
Source PublicationSolar RRL
ISSN2367-198X
Volume2Issue:2
Abstract

Solution-processed metal-halide perovskites have demonstrated immense potential in photovoltaic applications. Inkjet printing is a facile scalable approach to fabricate large-area perovskite solar cells (PSCs) due to its cost-effectiveness and near unity material utilization ratio. However, controlling crystallinity of the perovskite during the inkjet printing remains a challenge. The PSCs deposited by inkjet printing typically have much lower power conversion efficiencies (PCEs) than those by spin-coating. Here, we show that high-quality perovskite films could be inkjet-printed with an innovative vacuum-assisted thermal annealing post-treatment and optimized solvent composition. High-performance PSCs based on printed CHNHPbI with a PCE of 17.04% for 0.04 cm (13.27% for 4.0 cm) and negligible hysteresis (lower than 1.0%) are demonstrated. These efficiencies are much higher than the previously reported ones using inkjet-printing (≤12.3% for 0.04 cm). The inkjet printing combined with vacuum-assisted thermal annealing could be an effective low-cost approach to fabricate high-performance perovskite optoelectronic thin film devices (including solar cells, lasers, photodetectors, and light-emitting diodes) with high-volume production.

KeywordDroplet Manipulation Large-area Perovskite Solar Cells One-step Inkjet Printing Vacuum-assisted Thermal Annealing
DOI10.1002/solr.201700217
URLView the original
Indexed BySCIE
Language英語English
WOS Research AreaEnergy & Fuels ; Materials Science
WOS SubjectEnergy & Fuels ; Materials Science, Multidisciplinary
WOS IDWOS:000424658200009
Scopus ID2-s2.0-85077057977
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Document TypeJournal article
CollectionINSTITUTE OF APPLIED PHYSICS AND MATERIALS ENGINEERING
Corresponding AuthorZhang,Yiqiang; Xing,Guichuan
Affiliation1.State Centre for International Cooperation on Designer Low-Carbon and Environmental Material (SCICDLCEM) School of Materials Science and Engineering Zhengzhou University,Zhengzhou,450001,China
2.Institute of Applied Physics and Materials Engineering,University of Macau,999078,Macao
3.School of Materials Science and Engineering,Nanyang Technological University,Singapore,Nanyang Avenue,639798,Singapore
4.Key Laboratory of Green Printing,Institute of Chemistry,Chinese Academy of Sciences (ICCAS),Beijing Engineering Research Center of Nanomaterials for Green Printing Technology,Beijing National Laboratory for Molecular Sciences (BNLMS),Beijing,100190,China
Corresponding Author AffilicationINSTITUTE OF APPLIED PHYSICS AND MATERIALS ENGINEERING
Recommended Citation
GB/T 7714
Liang,Chao,Li,Pengwei,Gu,Hao,et al. One-Step Inkjet Printed Perovskite in Air for Efficient Light Harvesting[J]. Solar RRL, 2018, 2(2).
APA Liang,Chao., Li,Pengwei., Gu,Hao., Zhang,Yiqiang., Li,Fengyu., Song,Yanlin., Shao,Guosheng., Mathews,Nripan., & Xing,Guichuan (2018). One-Step Inkjet Printed Perovskite in Air for Efficient Light Harvesting. Solar RRL, 2(2).
MLA Liang,Chao,et al."One-Step Inkjet Printed Perovskite in Air for Efficient Light Harvesting".Solar RRL 2.2(2018).
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