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Size-Controlled Patterning of Single-Crystalline Perovskite Arrays toward a Tunable High-Performance Microlaser
Du,Huigang1; Wang,Kaiyang3; Zhao,Lidan1; Xue,Chang1; Zhang,Mengying2; Wen,Weijia1,4; Xing,Guichuan3; Wu,Jinbo1
2019-12-19
Source PublicationACS Applied Materials and Interfaces
ISSN1944-8244
Volume12Issue:2Pages:2662-2670
Abstract

Single-crystalline halide perovskites with regular morphology are of great significance for laser applications because they can be used to fabricate a natural whispering-gallery-mode resonator. Although enormous efforts have been put to synthesize single-crystalline perovskites, controlling the lateral size and thickness of the crystal, particularly at the nanoscale, is still challenging. Here, we report a facile and high-throughput strategy to selectively one-step create micro/nanoscale size-controlled all-inorganic perovskite single-crystal arrays by surface-tension-confined evaporative assembly. Our method can be used to easily tune the single crystal size and selectively position the single crystal, with versatility in fabricating perovskite single-crystal arrays in a wafer scale. When the patterned size increases from 2 to 25 μm, the width of the CsPbClBr perovskite microplates increased from 150 nm to 4.2 μm. Fixing the width of the microplates at 1.6 μm, with the increase of the sliding speed from 50 to 250 mm/min, we could significantly control the thicknesses from 270 to 430 nm. Additionally, our present study provides a characterization of lasers based on different three-dimensional structures, confirming their width-dependent lasing mode and thickness-dependent lasing threshold characteristic, which is beneficial for the tunability of a high-performance microlaser.

KeywordEvaporative Assembly Halide-perovskite Microlaser Single Crystal Surface-tension-confined
DOI10.1021/acsami.9b18512
URLView the original
Indexed BySCIE
Language英語English
WOS Research AreaScience & Technology - Other Topics ; Materials Science
WOS SubjectNanoscience & Nanotechnology ; Materials Science, Multidisciplinary
WOS IDWOS:000508464500076
PublisherAMER CHEMICAL SOC, 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
Scopus ID2-s2.0-85077952627
Fulltext Access
Citation statistics
Document TypeJournal article
CollectionINSTITUTE OF APPLIED PHYSICS AND MATERIALS ENGINEERING
Corresponding AuthorWu,Jinbo
Affiliation1.Materials Genome Institute,Shanghai University,Shanghai,200444,China
2.Department of Physics,Shanghai University,Shanghai,200444,China
3.Joint Key Laboratory of the Ministry of Education,Institute of Applied Physics and Materials Engineering,University of Macau,Taipa,Avenida da Universidade,999078,Macao
4.Department of Physics,Hong Kong University of Science and Technology,Kowloon,999077,Hong Kong
Recommended Citation
GB/T 7714
Du,Huigang,Wang,Kaiyang,Zhao,Lidan,et al. Size-Controlled Patterning of Single-Crystalline Perovskite Arrays toward a Tunable High-Performance Microlaser[J]. ACS Applied Materials and Interfaces, 2019, 12(2), 2662-2670.
APA Du,Huigang., Wang,Kaiyang., Zhao,Lidan., Xue,Chang., Zhang,Mengying., Wen,Weijia., Xing,Guichuan., & Wu,Jinbo (2019). Size-Controlled Patterning of Single-Crystalline Perovskite Arrays toward a Tunable High-Performance Microlaser. ACS Applied Materials and Interfaces, 12(2), 2662-2670.
MLA Du,Huigang,et al."Size-Controlled Patterning of Single-Crystalline Perovskite Arrays toward a Tunable High-Performance Microlaser".ACS Applied Materials and Interfaces 12.2(2019):2662-2670.
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