Residential College | false |
Status | 已發表Published |
Size-Controlled Patterning of Single-Crystalline Perovskite Arrays toward a Tunable High-Performance Microlaser | |
Du,Huigang1; Wang,Kaiyang3; Zhao,Lidan1; Xue,Chang1; Zhang,Mengying2; Wen,Weijia1,4; Xing,Guichuan3; Wu,Jinbo1 | |
2019-12-19 | |
Source Publication | ACS Applied Materials and Interfaces |
ISSN | 1944-8244 |
Volume | 12Issue:2Pages:2662-2670 |
Abstract | Single-crystalline halide perovskites with regular morphology are of great significance for laser applications because they can be used to fabricate a natural whispering-gallery-mode resonator. Although enormous efforts have been put to synthesize single-crystalline perovskites, controlling the lateral size and thickness of the crystal, particularly at the nanoscale, is still challenging. Here, we report a facile and high-throughput strategy to selectively one-step create micro/nanoscale size-controlled all-inorganic perovskite single-crystal arrays by surface-tension-confined evaporative assembly. Our method can be used to easily tune the single crystal size and selectively position the single crystal, with versatility in fabricating perovskite single-crystal arrays in a wafer scale. When the patterned size increases from 2 to 25 μm, the width of the CsPbClBr perovskite microplates increased from 150 nm to 4.2 μm. Fixing the width of the microplates at 1.6 μm, with the increase of the sliding speed from 50 to 250 mm/min, we could significantly control the thicknesses from 270 to 430 nm. Additionally, our present study provides a characterization of lasers based on different three-dimensional structures, confirming their width-dependent lasing mode and thickness-dependent lasing threshold characteristic, which is beneficial for the tunability of a high-performance microlaser. |
Keyword | Evaporative Assembly Halide-perovskite Microlaser Single Crystal Surface-tension-confined |
DOI | 10.1021/acsami.9b18512 |
URL | View the original |
Indexed By | SCIE |
Language | 英語English |
WOS Research Area | Science & Technology - Other Topics ; Materials Science |
WOS Subject | Nanoscience & Nanotechnology ; Materials Science, Multidisciplinary |
WOS ID | WOS:000508464500076 |
Publisher | AMER CHEMICAL SOC, 1155 16TH ST, NW, WASHINGTON, DC 20036 USA |
Scopus ID | 2-s2.0-85077952627 |
Fulltext Access | |
Citation statistics | |
Document Type | Journal article |
Collection | INSTITUTE OF APPLIED PHYSICS AND MATERIALS ENGINEERING |
Corresponding Author | Wu,Jinbo |
Affiliation | 1.Materials Genome Institute,Shanghai University,Shanghai,200444,China 2.Department of Physics,Shanghai University,Shanghai,200444,China 3.Joint Key Laboratory of the Ministry of Education,Institute of Applied Physics and Materials Engineering,University of Macau,Taipa,Avenida da Universidade,999078,Macao 4.Department of Physics,Hong Kong University of Science and Technology,Kowloon,999077,Hong Kong |
Recommended Citation GB/T 7714 | Du,Huigang,Wang,Kaiyang,Zhao,Lidan,et al. Size-Controlled Patterning of Single-Crystalline Perovskite Arrays toward a Tunable High-Performance Microlaser[J]. ACS Applied Materials and Interfaces, 2019, 12(2), 2662-2670. |
APA | Du,Huigang., Wang,Kaiyang., Zhao,Lidan., Xue,Chang., Zhang,Mengying., Wen,Weijia., Xing,Guichuan., & Wu,Jinbo (2019). Size-Controlled Patterning of Single-Crystalline Perovskite Arrays toward a Tunable High-Performance Microlaser. ACS Applied Materials and Interfaces, 12(2), 2662-2670. |
MLA | Du,Huigang,et al."Size-Controlled Patterning of Single-Crystalline Perovskite Arrays toward a Tunable High-Performance Microlaser".ACS Applied Materials and Interfaces 12.2(2019):2662-2670. |
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