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Stable Whispering Gallery Mode Lasing from Solution-Processed Formamidinium Lead Bromide Perovskite Microdisks
Xiaojun Li1; Kaiyang Wang1; Mingming Chen2; Sisi Wang1; Yubin Fan3; Tao Liang1; Qinghai Song3; Guichuan Xing1; Zikang Tang1
2020-08
Source PublicationAdvanced Optical Materials
ISSN2195-1071
Volume8Issue:15Pages:2000030
Other Abstract

Formamidinium (CH(NH2)2, FA) lead halide perovskites exhibit excellent optoelectronic properties for the applications of light-emitting diodes and lasers. However, the reported formamidinium lead bromide (FAPbBr3) perovskite-based lasers mainly depend on the external feedback or Fabry–Pérot mode cavities and suffer from moderate quality (Q) factors. Herein, solution-processed square and quasi-circular FAPbBr3 microdisks are developed to achieve room-temperature naturally facet-formed whispering gallery mode (WGM) lasers. These microdisks exhibit relatively high Q factor and tunable laser modes with threshold of 10–70 µJ cm−2 under 400 nm excitation. Although the synthesized circular microdisk is not regular enough, it still shows higher Q factor of 3455 than that of square microdisk due to the less boundary wave and pesudointegrable leakage. This simple and low-cost solution processed method can tackle the complicated and expensive conventional preparation techniques of circular microdisks. Power dependent photoluminescence decay transients indicate that the band edge emission of the FAPbBr3 microdisks originates from free carrier recombination. In addition, these microdisks show high photostability and that room temperature lasing can sustain over 50 min. These results suggest that FAPbBr3 microdisks can serve as promising WGM lasers with excellent light emission capability and stability toward practical optoelectronic applications.

DOI10.1002/adom.202000030
URLView the original
Indexed BySCIE
Language英語English
WOS Research AreaMaterials Science ; Optics
WOS SubjectMaterials Science, Multidisciplinary ; Optics
WOS IDWOS:000531269300001
PublisherWILEY-V C H VERLAG GMBH, POSTFACH 101161, 69451 WEINHEIM, GERMANY
Scopus ID2-s2.0-85085151696
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Citation statistics
Document TypeJournal article
CollectionINSTITUTE OF APPLIED PHYSICS AND MATERIALS ENGINEERING
Corresponding AuthorGuichuan Xing; Zikang Tang
Affiliation1.Institute of Applied Physics and Materials Engineering,University of Macau,Avenida da Universidade,Taipa,999078,Macao
2.Department of Physics,Jiangsu University,Zhenjiang,212013,China
3.State Key Laboratory on Tunable laser Technology,Ministry of Industry and Information Technology Key Lab of Micro-Nano Optoelectronic Information System,Shenzhen Graduate School,Harbin Institute of Technology,Shenzhen,518055,China
First Author AffilicationINSTITUTE OF APPLIED PHYSICS AND MATERIALS ENGINEERING
Corresponding Author AffilicationINSTITUTE OF APPLIED PHYSICS AND MATERIALS ENGINEERING
Recommended Citation
GB/T 7714
Xiaojun Li,Kaiyang Wang,Mingming Chen,et al. Stable Whispering Gallery Mode Lasing from Solution-Processed Formamidinium Lead Bromide Perovskite Microdisks[J]. Advanced Optical Materials, 2020, 8(15), 2000030.
APA Xiaojun Li., Kaiyang Wang., Mingming Chen., Sisi Wang., Yubin Fan., Tao Liang., Qinghai Song., Guichuan Xing., & Zikang Tang (2020). Stable Whispering Gallery Mode Lasing from Solution-Processed Formamidinium Lead Bromide Perovskite Microdisks. Advanced Optical Materials, 8(15), 2000030.
MLA Xiaojun Li,et al."Stable Whispering Gallery Mode Lasing from Solution-Processed Formamidinium Lead Bromide Perovskite Microdisks".Advanced Optical Materials 8.15(2020):2000030.
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