Residential College | false |
Status | 已發表Published |
Solution‐Processed Perovskite Microdisk for Coherent Light Emission | |
Xiaojun Li1; Xuanjun Zhang2; Haifeng Li1; Tanghao Liu1; Dandan Zhao1; Chao Liang1; Guichuan Xing1; Zikang Tang1 | |
2019-10 | |
Source Publication | ADVANCED OPTICAL MATERIALS |
ISSN | 2195-1071 |
Volume | 7Issue:19 |
Other Abstract | High‐quality semiconductor microdisks (MDs) are of crucial importance for realizing on‐chip coherent light sources. However, the fabrication of all‐inorganic semiconductor circular or circular‐like microdisks (CMDs) with suitable size for optoelectronic applications is still complex and expensive. Herein, a facile ligand‐free antisolvent‐assisted growth method is used to synthesize high‐quality Cs4PbBr6 MDs with tunable size and morphology, which is evolved from rhombohedral to octahedral, hexagonal‐like, and circular‐like MDs based on Cl‐containing antisolvents. Significantly, this is the first time that large semiconductor CMDs are synthesized from solution self‐assembled growth at room temperature. These Cs4PbBr6 MDs show high‐efficient and stable green emission (522 nm), which should be attributed to the first‐order excitonic emission from embedded CsPbBr3 nanocrystals (NCs). The distribution of CsPbBr3 NCs is verified by lattice fringe, crystal data refinement, and time‐resolved photoluminescence analysis. These CsPbBr3‐in‐Cs4PbBr6 CMDs are demonstrated to hold outstanding two‐photon pumped coherent light emission ability with a remarkably low threshold (400 µJ cm−2). These findings suggest CsPbBr3‐in‐Cs4PbBr6 MDs have excellent light emission capability and stability toward practical optoelectronic applications, and their tunable morphology and size indicate that solution method is feasible for the fabrication of semiconductor CMDs. |
DOI | 10.1002/adom.201900678 |
Indexed By | SCIE |
Language | 英語English |
WOS Research Area | Materials Science ; Optics |
WOS Subject | Materials Science, Multidisciplinary ; Optics |
WOS ID | WOS:000473950600001 |
Publisher | WILEY-V C H VERLAG GMBH, POSTFACH 101161, 69451 WEINHEIM, GERMANY |
Scopus ID | 2-s2.0-85068474087 |
Fulltext Access | |
Citation statistics | |
Document Type | Journal article |
Collection | INSTITUTE OF APPLIED PHYSICS AND MATERIALS ENGINEERING Faculty of Health Sciences |
Corresponding Author | Guichuan Xing; Zikang Tang |
Affiliation | 1.Joint Key Laboratory of the Ministry of Education, Institute of Applied Physics and Materials Engineering, University of Macau, Avenida da Universidade, Taipa, Macau SAR, 999078 China 2.Faculty of Health Sciences, University of Macau, Avenida da Universidade, Taipa, Macau SAR, 999078 China |
First Author Affilication | INSTITUTE OF APPLIED PHYSICS AND MATERIALS ENGINEERING |
Corresponding Author Affilication | INSTITUTE OF APPLIED PHYSICS AND MATERIALS ENGINEERING |
Recommended Citation GB/T 7714 | Xiaojun Li,Xuanjun Zhang,Haifeng Li,et al. Solution‐Processed Perovskite Microdisk for Coherent Light Emission[J]. ADVANCED OPTICAL MATERIALS, 2019, 7(19). |
APA | Xiaojun Li., Xuanjun Zhang., Haifeng Li., Tanghao Liu., Dandan Zhao., Chao Liang., Guichuan Xing., & Zikang Tang (2019). Solution‐Processed Perovskite Microdisk for Coherent Light Emission. ADVANCED OPTICAL MATERIALS, 7(19). |
MLA | Xiaojun Li,et al."Solution‐Processed Perovskite Microdisk for Coherent Light Emission".ADVANCED OPTICAL MATERIALS 7.19(2019). |
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