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High brightness formamidinium lead bromide perovskite nanocrystal light emitting devices
Perumal A.1; Shendre S.1; Li M.1; Tay Y.K.E.1; Sharma V.K.1; Chen S.1; Wei Z.1; Liu Q.1; Gao Y.1; Buenconsejo P.J.S.1; Tan S.T.1; Gan C.L.1; Xiong Q.1; Sum T.C.1; Demir H.V.1
2016-11-09
Source PublicationScientific Reports
ISSN20452322
Volume6
Abstract

Formamidinium lead halide (FAPbX) has attracted greater attention and is more prominent recently in photovoltaic devices due to its broad absorption and higher thermal stability in comparison to more popular methylammonium lead halide MAPbX. Herein, a simple and highly reproducible room temperature synthesis of device grade high quality formamidinium lead bromide CH(NH) PbBr (FAPbBr) colloidal nanocrystals (NC) having high photoluminescence quantum efficiency (PLQE) of 55-65% is reported. In addition, we demonstrate high brightness perovskite light emitting device (Pe-LED) with these FAPbBr perovskite NC thin film using 2,2′,2″-(1,3,5-Benzinetriyl)-tris(1-phenyl-1-H-benzimidazole) commonly known as TPBi and 4,6-Bis(3,5-di(pyridin-3-yl)phenyl)-2-methylpyrimidine (B3PYMPM) as electron transport layers (ETL). The Pe-LED device with B3PYMPM as ETL has bright electroluminescence of up to 2714 cd/m, while the Pe-LED device with TPBi as ETL has higher peak luminous efficiency of 6.4 cd/A and peak luminous power efficiency of 5.7 lm/W. To our knowledge this is the first report on high brightness light emitting device based on CH(NH) PbBr widely known as FAPbBr nanocrystals in literature.

DOI10.1038/srep36733
URLView the original
Language英語English
WOS IDWOS:000387542500001
Scopus ID2-s2.0-84994495769
Fulltext Access
Citation statistics
Document TypeJournal article
CollectionUniversity of Macau
Affiliation1.Nanyang Technological University
2.Bilkent Üniversitesi
Recommended Citation
GB/T 7714
Perumal A.,Shendre S.,Li M.,et al. High brightness formamidinium lead bromide perovskite nanocrystal light emitting devices[J]. Scientific Reports, 2016, 6.
APA Perumal A.., Shendre S.., Li M.., Tay Y.K.E.., Sharma V.K.., Chen S.., Wei Z.., Liu Q.., Gao Y.., Buenconsejo P.J.S.., Tan S.T.., Gan C.L.., Xiong Q.., Sum T.C.., & Demir H.V. (2016). High brightness formamidinium lead bromide perovskite nanocrystal light emitting devices. Scientific Reports, 6.
MLA Perumal A.,et al."High brightness formamidinium lead bromide perovskite nanocrystal light emitting devices".Scientific Reports 6(2016).
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