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Van der Waals integration of phase-pure 2D perovskite sheets and GaAs nanowires for self-driven photodetector
Zhang, Zhi Hong1,2; Hou, Xiao Bing1; Li, Shang Heng1; Wei, Zhi Peng1; Wei, Jin Chao3; Li, Peng3; Wang, Shuang Peng2
2024-09-26
Source PublicationJournal of Materials Chemistry C
ISSN2050-7526
Volume12Issue:37Pages:15232–15238
Abstract

Semiconductor heterostructures hold significant importance for exploring novel functional optoelectronic devices, but the chemical instability and soft lattice framework of perovskites significantly hinder the efficient heterogeneous integration with other perovskite or semiconductor materials. Herein, based on the large-area phase-pure 2D perovskite sheets, a BAMAPbI/GaAs van der Waals (vdW) heterostructure has been successfully constructed. The favorable vdW contacts allow the device to be cut-off at forward bias with a remarkably low dark current of 1.94 pA. This endows the heterostructure device with excellent detection performance, achieving a linear dynamic range of 80.9 dB and a detectivity of 6.17 × 10 Jones. Additionally, the interfacial potential of the heterostructure enables the device to operate in a self-driven manner across broad spectral ranges from ultraviolet to near-infrared. Our study demonstrates efficient vdW integration based on perovskite and provides a new foundation for constructing perovskite vdW heterostructures.

DOI10.1039/d4tc02994a
URLView the original
Indexed BySCIE
Language英語English
WOS Research AreaMaterials Science Physics
WOS SubjectMaterials Science, Multidisciplinary Physics ; Applied
WOS IDWOS:001303429500001
PublisherROYAL SOC CHEMISTRY, THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS, ENGLAND
Scopus ID2-s2.0-85202996411
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Citation statistics
Document TypeJournal article
CollectionInstitute of Chinese Medical Sciences
INSTITUTE OF APPLIED PHYSICS AND MATERIALS ENGINEERING
Corresponding AuthorWei, Zhi Peng; Wang, Shuang Peng
Affiliation1.State Key Laboratory of High Power Semiconductor Lasers, Changchun University of Science and Technology, Changchun, 130022, China
2.Institute of Applied Physics and Materials Engineering, University of Macau, Taipa, Macao SAR, 999078, Macao
3.State Key Laboratory of Quality Research in Chinese Medicine, Institute of Chinese Medical Sciences, University of Macau, Macau, 999078, Macao
First Author AffilicationINSTITUTE OF APPLIED PHYSICS AND MATERIALS ENGINEERING
Corresponding Author AffilicationINSTITUTE OF APPLIED PHYSICS AND MATERIALS ENGINEERING
Recommended Citation
GB/T 7714
Zhang, Zhi Hong,Hou, Xiao Bing,Li, Shang Heng,et al. Van der Waals integration of phase-pure 2D perovskite sheets and GaAs nanowires for self-driven photodetector[J]. Journal of Materials Chemistry C, 2024, 12(37), 15232–15238.
APA Zhang, Zhi Hong., Hou, Xiao Bing., Li, Shang Heng., Wei, Zhi Peng., Wei, Jin Chao., Li, Peng., & Wang, Shuang Peng (2024). Van der Waals integration of phase-pure 2D perovskite sheets and GaAs nanowires for self-driven photodetector. Journal of Materials Chemistry C, 12(37), 15232–15238.
MLA Zhang, Zhi Hong,et al."Van der Waals integration of phase-pure 2D perovskite sheets and GaAs nanowires for self-driven photodetector".Journal of Materials Chemistry C 12.37(2024):15232–15238.
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