Residential College | false |
Status | 已發表Published |
Highly-Entangled Hydrogel Electrolyte for Fast Charging/Discharging Properties in Aqueous Zinc Ion Batteries | |
Shen, Zhaoxi1; Liu, Yu2; Li, Zhongheng2; Tang, Ziqing3; Pu, Jun4; Luo, Lei2; Ji, Yu2; Xie, Junpeng5; Shu, Zheng2; Yao, Yagang4; Zhang, Ning1; Hong, Guo5 | |
2024-07 | |
Source Publication | Advanced Functional Materials |
ISSN | 1616-301X |
Pages | 2406620 |
Abstract | Aqueous zinc ion batteries coupling with conventional hydrogel electrolyte have the advantages of high safety, low cost, and simple manufacturing process while they are difficult for fast charging/discharging application scenarios due to the sluggish kinetics. Herein, a new strategy is developed for synthesizing a highly-entangled polyacrylamide (HE-PAM) hydrogel electrolyte to dramatically enhance the ion transportation and mechanical stability. The developed hydrogel electrolyte has lower ionic resistance and a strong elastic modulus. After being assembled into Zn/MnO2 batteries, the HE-PAM hydrogel electrolyte exhibits excellent cycling stability and high-rate capability under high current densities. Specifically, the Zn//HE-PAM//MnO2 battery can resist the highest current of 35 Ag-1, which outperforms previously reported works. Moreover, the HE-PAM hydrogel electrolyte can also support the fast charging/discharging in proton ion batteries with a high capacity retention rate of 50% under 50 Ag-1. This progress on hydrogel electrolytes can boost the development of quasi-solid-state batteries in the fast charging/discharging aspect. |
Keyword | Fast Charging/discharging Highly-entangled Polyacrylamide Hydrogel Electrolyte Proton Ion Batteries Zn/mno2 Batteries |
DOI | 10.1002/adfm.202406620 |
URL | View the original |
Indexed By | SCIE |
Language | 英語English |
WOS Research Area | Chemistry ; Science & Technology - Other Topics ; Materials Science ; Physics |
WOS Subject | Chemistry, Multidisciplinary ; Chemistry, Physical ; Nanoscience & Nanotechnology ; Materials Science, Multidisciplinary ; Physics, Applied ; Physics, Condensed Matter |
WOS ID | WOS:001263080700001 |
Publisher | WILEY-V C H VERLAG GMBH, POSTFACH 101161, 69451 WEINHEIM, GERMANY |
Scopus ID | 2-s2.0-85197874614 |
Fulltext Access | |
Citation statistics | |
Document Type | Journal article |
Collection | INSTITUTE OF APPLIED PHYSICS AND MATERIALS ENGINEERING |
Corresponding Author | Zhang, Ning; Hong, Guo |
Affiliation | 1.College of Chemistry and Materials Science, Key Laboratory of Analytical Science and Technology of Hebei Province, Institute of Life Science and Green Development, Hebei University, Baoding, 071002, China 2.Institute of Applied Physics and Materials Engineering, University of Macau, Avenida da Universidade, Taipa, 999078, Macao 3.Wenzhou Institute, University of Chinese Academy of Sciences, Wenzhou, 352001, China 4.National Laboratory of Solid State Microstructures, College of Engineering and Applied Sciences, Jiangsu Key Laboratory of Artificial Functional Materials, Collaborative Innovation Center of Advanced Microstructures, Nanjing University 5.Department of Materials Science and Engineering & Centre of Super-Diamond and Advanced Films (COSDAF), City University of Hong Kong, Kowloon, 999077, Hong Kong |
Recommended Citation GB/T 7714 | Shen, Zhaoxi,Liu, Yu,Li, Zhongheng,et al. Highly-Entangled Hydrogel Electrolyte for Fast Charging/Discharging Properties in Aqueous Zinc Ion Batteries[J]. Advanced Functional Materials, 2024, 2406620. |
APA | Shen, Zhaoxi., Liu, Yu., Li, Zhongheng., Tang, Ziqing., Pu, Jun., Luo, Lei., Ji, Yu., Xie, Junpeng., Shu, Zheng., Yao, Yagang., Zhang, Ning., & Hong, Guo (2024). Highly-Entangled Hydrogel Electrolyte for Fast Charging/Discharging Properties in Aqueous Zinc Ion Batteries. Advanced Functional Materials, 2406620. |
MLA | Shen, Zhaoxi,et al."Highly-Entangled Hydrogel Electrolyte for Fast Charging/Discharging Properties in Aqueous Zinc Ion Batteries".Advanced Functional Materials (2024):2406620. |
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