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Electrical control of excitonic oscillator strength and spatial distribution in a monolayer semiconductor
Wang, Yanming1,2; Zhang, Junrong1,2; Ren, Tianhua3; Xia, Meng2; Fang, Long2,4; Wang, Xiangyi2; Zhang, Xingwang1,2; Zhang, Kai1,2; Wang, Junyong1,2
2024-09
Source PublicationNano Research
ISSN1998-0124
Volume17Issue:9Pages:8424-8430
Abstract

Electrical modulation of luminescence is significant to modern light-emitting devices. Monolayer transition metal dichalcogenides are emerging direct-bandgap luminescent materials with unique excitonic properties, and the multiple exciton complexes provide new opportunities to modulate the property of luminescence in atomically thin semiconductors. Here, we report an electrical control of exciton emission in the oscillator strength and spatial distribution of excitons in a monolayer WS. Effective modulation of excitonic emission intensity with a degree of modulation of ~ 92% has been demonstrated by an electric field at room temperature. The spatial carrier redistribution tuned by a lateral electric field results in distinct excitonic emission patterns by design. The modulation approach to exciton oscillator strength and distribution provides an efficient way to investigate the exciton diffusion dynamics and to construct electrically tunable optoelectronic devices.

KeywordElectrical Modulation Exciton Monolayer Semiconductor Spatial Distribution
DOI10.1007/s12274-024-6762-7
URLView the original
Indexed BySCIE
Language英語English
WOS Research AreaChemistry ; Science & Technology - Other Topics ; Materials Science ; Physics
WOS SubjectChemistry, Physical ; Nanoscience & Nanotechnology ; Materials Science, Multidisciplinary ; Physics, Applied
WOS IDWOS:001261260500002
PublisherTSINGHUA UNIV PRESS, B605D, XUE YAN BUILDING, BEIJING 100084, PEOPLES R CHINA
Scopus ID2-s2.0-85198518321
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Citation statistics
Document TypeJournal article
CollectionINSTITUTE OF APPLIED PHYSICS AND MATERIALS ENGINEERING
Corresponding AuthorZhang, Kai; Wang, Junyong
Affiliation1.School of Nano-Tech and Nano-Bionics, University of Science and Technology of China, Hefei, 230026, China
2.CAS Key Laboratory of Nanophotonic Materials and Devices & amp; Key Laboratory of Nanodevices and Applications, i-Lab, Suzhou Institute of Nano-Tech and Nano-Bionics (SINANO), Chinese Academy of Sciences, Suzhou, 215123, China
3.Institute of Applied Physics and Materials Engineering, University of Macau, Taipa, 999078, Macao
4.College of New Energy, Inner Mongolia University of Technology, Hohhot, 010051, China
Recommended Citation
GB/T 7714
Wang, Yanming,Zhang, Junrong,Ren, Tianhua,et al. Electrical control of excitonic oscillator strength and spatial distribution in a monolayer semiconductor[J]. Nano Research, 2024, 17(9), 8424-8430.
APA Wang, Yanming., Zhang, Junrong., Ren, Tianhua., Xia, Meng., Fang, Long., Wang, Xiangyi., Zhang, Xingwang., Zhang, Kai., & Wang, Junyong (2024). Electrical control of excitonic oscillator strength and spatial distribution in a monolayer semiconductor. Nano Research, 17(9), 8424-8430.
MLA Wang, Yanming,et al."Electrical control of excitonic oscillator strength and spatial distribution in a monolayer semiconductor".Nano Research 17.9(2024):8424-8430.
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