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Hyperbolic response and low-frequency ultra-flat plasmons in inhomogeneous charge-distributed transition-metal monohalides
Han, G. A.O.1,2; Ning, Q. U.1; Zhang, Xuejin3; Ding, Chao2; Wang, Mingzheng2; Wang, Juan4; Yang, Bo1; Zhao, Mingwen2
2024-06-17
Source PublicationOptics Express
ISSN1094-4087
Volume32Issue:13Pages:22525-22536
Abstract

Plasmon, the collective oscillations of free electron gas in materials, determines the long-wavelength excitation spectrum and optical response, are pivotal in the realm of nanophotonics and optoelectronics. In this study, using the first-principles calculations, we systematically investigated the dielectric response and plasmon properties of bulk transition-metal monohalides MXs (M = Zr, Mo; X = Cl, F). Due to the strong electronic anisotropy, MXs exhibit a broadband type-II hyperbolic response and direction-dependent plasmon modes. Particularly, local field effect (LFE) driven by the charge distribution inhomogeneity, significantly modifies the optical response and excitation spectra in MX along the out-of-plane direction. Taking into account LFE, the energy dissipation along the out-of-plane direction is almost completely suppressed, and an ultra-flat and long-lived plasmon mode with a slow group velocity is introduced. This finding reveals the role of charge density in modifying the optical response and excitation behavior, shedding light on potential applications in plasmonics.

KeywordDielectric-constant Density-wave Dispersion Energy Excitations Polaritons Solar Zirconium Scattering
DOI10.1364/OE.524893
URLView the original
Indexed BySCIE
Language英語English
WOS Research AreaOptics
WOS SubjectOptics
WOS IDWOS:001253344700001
PublisherOptica Publishing Group, 2010 MASSACHUSETTS AVE NW, WASHINGTON, DC 20036
Scopus ID2-s2.0-85196751924
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Citation statistics
Document TypeJournal article
CollectionINSTITUTE OF APPLIED PHYSICS AND MATERIALS ENGINEERING
University of Macau
Corresponding AuthorHan, G. A.O.
Affiliation1.School of Science, Shandong Jianzhu University, Jinan, 250100, China
2.School of Physics, Shandong University, Jinan, 250100, China
3.Institute of Applied Physics and Materials Engineering, University of Macau, 519000, Macao
4.School of Physics and Electronic Engineering, Qilu Normal University, Jinan, 250200, China
Recommended Citation
GB/T 7714
Han, G. A.O.,Ning, Q. U.,Zhang, Xuejin,et al. Hyperbolic response and low-frequency ultra-flat plasmons in inhomogeneous charge-distributed transition-metal monohalides[J]. Optics Express, 2024, 32(13), 22525-22536.
APA Han, G. A.O.., Ning, Q. U.., Zhang, Xuejin., Ding, Chao., Wang, Mingzheng., Wang, Juan., Yang, Bo., & Zhao, Mingwen (2024). Hyperbolic response and low-frequency ultra-flat plasmons in inhomogeneous charge-distributed transition-metal monohalides. Optics Express, 32(13), 22525-22536.
MLA Han, G. A.O.,et al."Hyperbolic response and low-frequency ultra-flat plasmons in inhomogeneous charge-distributed transition-metal monohalides".Optics Express 32.13(2024):22525-22536.
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