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Pre-Lithiation Technology for Rechargeable Lithium-Ion Batteries: Principles, Applications, and Perspectives
Li, Shuang1; Jiang, Jiangmin1,2,3; Zheng, Yun2; Ju, Zhicheng1; Zhuang, Quanchao1; Wu, Kai1,4; Shao, Huaiyu2; Zhang, Xiaogang3
Source PublicationBATTERIES & SUPERCAPS
ISSN2566-6223
2024-03-24
Abstract

Lithium-ion batteries (LIBs) have been widely used as a new energy storage system with high energy density and long cycle life. However, the solid electrolyte interface (SEI) formed on the surface of anode consumes excess active lithium during the initial cycle, resulting in an initial irreversible capacity loss (ICL) and reducing the overall electrochemical performance. To solve the critical issue, pre-lithiation technology has been accepted as one of the most promising strategies. Due to the pre-lithiated treatment provides additional active lithium to compensate for the ICL and effectively improves initial Coulombic efficiency (ICE), leading to raising the working voltage, increasing the Li concentration, as well as improving the energy density and cycle stability of LIBs. In this overview, the causes of ICL in LIBs are analyzed from different perspectives, and various pre-lithiation strategies are systematically classified and summarized. Finally, some current problems and development prospects in this field are summarized, with prospects for realizing industrialized technologies.

KeywordCoulombic Efficiency Irreversible Capacity Loss Lithium-ion Batteries Pre-lithiation Technology Solid Electrolyte Interface
Language英語English
DOI10.1002/batt.202400115
URLView the original
Pagese202400115
WOS IDWOS:001207849300001
WOS SubjectElectrochemistry ; Materials Science, Multidisciplinary
WOS Research AreaElectrochemistry ; Materials Science
Indexed BySCIE
Scopus ID2-s2.0-85191242746
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Citation statistics
Document TypeReview article
CollectionINSTITUTE OF APPLIED PHYSICS AND MATERIALS ENGINEERING
Corresponding AuthorJiang, Jiangmin; Wu, Kai; Shao, Huaiyu; Zhang, Xiaogang
Affiliation1.Jiangsu Province Engineering Laboratory of High Efficient Energy Storage Technology and Equipments, School of Materials Science and Physics, China University of Mining and Technology, Xuzhou, 221116, China
2.Guangdong-Hong Kong-Macau Joint Laboratory for Photonic-Thermal-Electrical Energy Materials and Devices, Institute of Applied Physics and Materials Engineering, University of Macau, 999078, Macao
3.Jiangsu Key Laboratory of Electrochemical Energy Storage Technology, College of Material Science and Engineering, Nanjing University of Aeronautics and Astronautics, Nanjing, 210016, China
4.Contemporary Amperex Technology Co. Limited, Ningde, 352100, China
Corresponding Author AffilicationINSTITUTE OF APPLIED PHYSICS AND MATERIALS ENGINEERING
Recommended Citation
GB/T 7714
Li, Shuang,Jiang, Jiangmin,Zheng, Yun,et al. Pre-Lithiation Technology for Rechargeable Lithium-Ion Batteries: Principles, Applications, and Perspectives[J]. BATTERIES & SUPERCAPS, 2024, e202400115.
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