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The synthesis and tunable topological properties of Sm-doped (Bi, Sb)2Te2S crystal
Wu, Junjie1; Liu, Zhanfeng2; Wang, Yuanyuan3; Ma, Xiang1; Wang, Shasha1; Tan, Haige1; Wang, Changlong1; Li, Ruimin1; Huang, Lizhen1; Xi, Chuanying4; Lu, Yalin1; Sun, Zhe2; Yang, Shengyuan A.3; Xiang, Bin1
2024-06-25
Source PublicationJournal of Alloys and Compounds
ISSN0925-8388
Volume989Pages:174359
Abstract

Topological insulators exhibit Dirac points in their topological surface states, but often such Dirac points are far from the Fermi level and sometimes even reside outside the bulk band gap. Here, we report the synthesis of a new topological insulator material Sm-doped (Bi, Sb)TeS, which has its surface tunable Dirac point exposed within the bulk gap and close to the Fermi level at a minimal distance of 73 meV with a large tunability of 157 meV, as evidenced by angle-resolved photoemission spectroscopy. The compensation doping by Sm creates a nearly insulating bulk and triggers an interesting phenomenon of all-configuration negative magnetoresistance. This signals a nearly compensated state where the bulk transport is mainly via percolation through charge puddles. Our work offers a new material platform suitable for regulating the position of surface Dirac points and exploring unique physical properties of topological insulators.

KeywordArpes Negative Magnetoresistance Topological Material Tunable Dirac Point
DOI10.1016/j.jallcom.2024.174359
URLView the original
Indexed BySCIE
Language英語English
WOS Research AreaChemistry ; Materials Science ; Metallurgy & Metallurgical Engineering
WOS SubjectChemistry, Physical ; Materials Science, Multidisciplinary ; Metallurgy & Metallurgical Engineering
WOS IDWOS:001221004100001
PublisherELSEVIER SCIENCE SA, PO BOX 564, 1001 LAUSANNE, SWITZERLAND
Scopus ID2-s2.0-85189517498
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Citation statistics
Document TypeJournal article
CollectionINSTITUTE OF APPLIED PHYSICS AND MATERIALS ENGINEERING
Corresponding AuthorSun, Zhe; Yang, Shengyuan A.; Xiang, Bin
Affiliation1.Department of Materials Science & Engineering, CAS Key Lab of Materials for Energy Conversion, Anhui Laboratory of Advanced Photon Science and Technology, University of Science and Technology of China, Hefei, 230026, China
2.National Synchrotron Radiation Laboratory, CAS Center for Excellence in Nanoscience, University of Science and Technology of China, Hefei, 230029, China
3.Research Laboratory for Quantum Materials, IAPME, University of Macau, 519000, China
4.Anhui Province Key Laboratory of Condensed Matter Physics at Extreme Conditions, High Magnetic Field Laboratory, Hefei Institutes of Physical Sciences, Chinese Academy of Science, Hefei, 230031, China
Corresponding Author AffilicationUniversity of Macau
Recommended Citation
GB/T 7714
Wu, Junjie,Liu, Zhanfeng,Wang, Yuanyuan,et al. The synthesis and tunable topological properties of Sm-doped (Bi, Sb)2Te2S crystal[J]. Journal of Alloys and Compounds, 2024, 989, 174359.
APA Wu, Junjie., Liu, Zhanfeng., Wang, Yuanyuan., Ma, Xiang., Wang, Shasha., Tan, Haige., Wang, Changlong., Li, Ruimin., Huang, Lizhen., Xi, Chuanying., Lu, Yalin., Sun, Zhe., Yang, Shengyuan A.., & Xiang, Bin (2024). The synthesis and tunable topological properties of Sm-doped (Bi, Sb)2Te2S crystal. Journal of Alloys and Compounds, 989, 174359.
MLA Wu, Junjie,et al."The synthesis and tunable topological properties of Sm-doped (Bi, Sb)2Te2S crystal".Journal of Alloys and Compounds 989(2024):174359.
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