Residential College | false |
Status | 已發表Published |
Facile Hydrogels of AIEgens Applied as Reusable Sensors for In Situ and Early Warning of Metallic Corrosion | |
Honglei Guo1; Canjie Zhu1,2; Zihao Yuan1; Guang Huang1,3; Huansen Liang1; Chenxi Xiong1; Zhiyuan Feng1; Qiang Wei4; Guozhe Meng1 | |
2023-01-31 | |
Source Publication | ACS Applied Materials & Interfaces |
ISSN | 1944-8244 |
Volume | 15Issue:6Pages:8530-8536 |
Abstract | Early detection of metallic corrosion is one considerable method to reduce imperceptible disasters nowadays. Fluorescent coatings with high sensitivity and long lifetimes for use in the early detection of metallic corrosion are in high demand, but they are presently difficult to prepare. Inspired by the chameleon’s skin, which is capable of switching its color in different atmospheres sensitively and reversibly, we proposed herein a facile and universal all-in-one strategy of combining the fluorescent sensitivity and dynamic hydrogen bonds in a hydrogel to develop a reusable corrosion detection tape to cover metal surfaces. The fluorescent hydrogel tape was constructed using free radical copolymerization of monomers [hydroxyethyl methylacrylate (HEMA) and tetraphenylethene derivatives (TPEPy)]. Due to the aggregation-induced emission (AIE) behavior of TPEPy, the poly(HEMA-co-TPEPy) hydrogel is capable of monitoring the traces of corrosion via the release of ferric ions with a concentration as low as 10 M. Moreover, due to the dynamic hydrogen bonds of hydroxyethyl groups in hydrogel networks, the fluorescent hydrogel tape exhibited good adhesion and well reusability for over 10 applications to effectively warn against early corrosion of stainless steel. This non-destructive and reversible method of early corrosion detection can provide valuable signals when maintenance is needed before the metal suffers serious damage. |
Keyword | Hydrogel Early Warning Metallic Corrosion Aiegens Reusability |
DOI | 10.1021/acsami.2c21798 |
URL | View the original |
Indexed By | SCIE |
Language | 英語English |
WOS Research Area | Science & Technology - Other Topics ; Materials Science |
WOS Subject | Nanoscience & Nanotechnology ; Materials Science, Multidisciplinary |
Publisher | AMER CHEMICAL SOC, 1155 16TH ST, NW, WASHINGTON, DC 20036 |
Scopus ID | 2-s2.0-85147203682 |
Fulltext Access | |
Citation statistics | |
Document Type | Journal article |
Collection | Faculty of Science and Technology |
Corresponding Author | Honglei Guo; Qiang Wei; Guozhe Meng |
Affiliation | 1.School of Chemical Engineering and Technology, Sun Yat-sen University, Zhuhai, 519082, China 2.School of Materials Science and Engineering, Sun Yat-sen University, Guangzhou, 510006, China 3.Faculty of Science and Technology, University of Macau, Taipa, 999078, Macao 4.Ningbo Institute of Materials Technology and Engineering (NIMTE), Chinese Academy of Sciences (CAS), Ningbo, 315201, China |
Recommended Citation GB/T 7714 | Honglei Guo,Canjie Zhu,Zihao Yuan,et al. Facile Hydrogels of AIEgens Applied as Reusable Sensors for In Situ and Early Warning of Metallic Corrosion[J]. ACS Applied Materials & Interfaces, 2023, 15(6), 8530-8536. |
APA | Honglei Guo., Canjie Zhu., Zihao Yuan., Guang Huang., Huansen Liang., Chenxi Xiong., Zhiyuan Feng., Qiang Wei., & Guozhe Meng (2023). Facile Hydrogels of AIEgens Applied as Reusable Sensors for In Situ and Early Warning of Metallic Corrosion. ACS Applied Materials & Interfaces, 15(6), 8530-8536. |
MLA | Honglei Guo,et al."Facile Hydrogels of AIEgens Applied as Reusable Sensors for In Situ and Early Warning of Metallic Corrosion".ACS Applied Materials & Interfaces 15.6(2023):8530-8536. |
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