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Self-Intercalated Magnetic Heterostructures in 2D Chromium Telluride
Niu, Kangdi1,2; Qiu, Guotao3; Wang, Chuanshou1; Li, Daiyue1,2; Niu, Yutao4,5; Li, Songge1; Kang, Lixing5; Cai, Yongqing3; Han, Mengjiao6; Lin, Junhao1,2
2023-01
Source PublicationAdvanced Functional Materials
ISSN1616-301X
Volume33Issue:2Pages:2208528
Abstract

Emerging 2D magnetic heterojunctions attract substantial interest due to their potential applications in spintronics. Achieving magnetic phase engineering with structural integrity in 2D heterojunctions is of paramount importance for their magnetism manipulation. Herein, starting with chromium ditelluride (CrTe) as the backbone framework, various lateral and vertical magnetic heterojunctions are obtained via self-intercalated 2D chromium telluride (CrTe). A CrTe-CrTe lateral heterojunction prototype is demonstrated for the manipulation of magnetic moments under different magnitudes of magnetic excitation, showing a sharply stepped hysteresis loop with a dual spin-flip transition at high Curie temperatures up to 150 and 210 K by magneto-optical Kerr measurement. High-resolution scanning transmission electron microscopy and first-principles calculations reveal a preferred random location of Cr intercalants at the phase boundary, allowing lowering energy associated with crystal field splitting. The overall structural rigidity of chromium-telluride heterostructure with magnetic phase decoupled behaviors is promising for 2D spintronic devices.

KeywordChromium Telluride Cr-intercalation Magnetic Heterostructures
DOI10.1002/adfm.202208528
URLView the original
Indexed BySCIE
Language英語English
WOS Research AreaChemistry ; Science & Technology - Other Topics ; Materials Science ; Physics
WOS SubjectChemistry, Multidisciplinary ; Chemistry, Physical ; Nanoscience & Nanotechnology ; Materials Science, Multidisciplinary ; Physics, Applied ; Physics, Condensed Matter
WOS IDWOS:000876135700001
PublisherWILEY-V C H VERLAG GMBH, POSTFACH 101161, 69451 WEINHEIM, GERMANY
Scopus ID2-s2.0-85141163264
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Document TypeJournal article
CollectionINSTITUTE OF APPLIED PHYSICS AND MATERIALS ENGINEERING
Corresponding AuthorCai, Yongqing; Han, Mengjiao; Lin, Junhao
Affiliation1.Department of Physics, Southern University of Science and Technology, Shenzhen, 518055, China
2.Shenzhen Key Laboratory of Advanced Quantum Functional Materials and Devices, Southern University of Science and Technology, Shenzhen, 518055, China
3.Institute of Applied Physics and Materials Engineering, University of Macau, Taipa, 999078, Macao
4.School of Nano-Tech and Nano-Bionics, University of Science and Technology of China, Hefei, 230026, China
5.Key Laboratory of Multifunctional Nanomaterials and Smart Systems, Advanced Materials Division, Suzhou Institute of Nano-Tech and Nano-Bionics, Chinese Academy of Sciences, Suzhou, 215123, China
6.Songshan Lake Materials Laboratory, Dongguan, Guangdong, 523808, China
Corresponding Author AffilicationINSTITUTE OF APPLIED PHYSICS AND MATERIALS ENGINEERING
Recommended Citation
GB/T 7714
Niu, Kangdi,Qiu, Guotao,Wang, Chuanshou,et al. Self-Intercalated Magnetic Heterostructures in 2D Chromium Telluride[J]. Advanced Functional Materials, 2023, 33(2), 2208528.
APA Niu, Kangdi., Qiu, Guotao., Wang, Chuanshou., Li, Daiyue., Niu, Yutao., Li, Songge., Kang, Lixing., Cai, Yongqing., Han, Mengjiao., & Lin, Junhao (2023). Self-Intercalated Magnetic Heterostructures in 2D Chromium Telluride. Advanced Functional Materials, 33(2), 2208528.
MLA Niu, Kangdi,et al."Self-Intercalated Magnetic Heterostructures in 2D Chromium Telluride".Advanced Functional Materials 33.2(2023):2208528.
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