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Robust Ultralong Lead Halide Perovskite Microwire Lasers
Yan, S.S.1; Wang, K.Y.1; Xing, G.C.1; Xu, J.C.1; Su, S.C.2,3; Tang, Z.K.1; Wang, S.P.1; Ng, K.W.1
2021-08-01
Source PublicationACS Applied Material Interfaces
ISSN1944-8244 (print); 1944-8252 (web)
Volume13Issue:32Pages:38458-38466
Abstract

Hybrid organic–inorganic lead halide perovskite microwires are potential building blocks for realizing on-chip integrated optoelectronic devices. However, the length-controllable synthesis of one-dimensional hybrid perovskite microwires has been rarely reported, especially the ones with lengths in the millimeter scale. Herein, methylammonium lead bromide (MAPbBr3) and formamidinium lead bromide (FAPbBr3) micro and milliwires are demonstrated using single-crystal PbBr2 microwires synthesized via template-free solution-phase growth as the lattice framework. Following the PbBr2 template, the as-converted perovskite microwires possess controllable lengths ranging from tens to thousands of micrometers. In addition, Fabry–Perot (FP) lasing was realized in both MAPbBr3 and FAPbBr3 microwires, attesting to their excellent crystal quality and the efficient optical confinement of the natural cavity. These unique properties result in the first demonstration of FP perovskite microwire lasers with submillimeter lengths. More interestingly, the microwire lasers show excellent photostability under repetitive pulsed laser excitation for over 8 × 106 cycles. Such findings demonstrate that the solution-converted hybrid lead bromide microwires have excellent optoelectronic performances promising for practical applications, and the size controllability indicates that this novel fabrication process may be feasible for large-scale industrial production.

KeywordUltralong Perovskite Microwires Controllable Length Fp Lasing Photostability Thermal Stability
DOI10.1021/acsami.1c08287
URLView the original
Indexed BySCIE
Language英語English
WOS Research AreaScience & Technology - Other Topics ; Materials Science
WOS SubjectNanoscience & Nanotechnology ; Materials Science, Multidisciplinary
WOS IDWOS:000687172000051
PublisherAMER CHEMICAL SOC1155 16TH ST, NW, WASHINGTON, DC 20036
The Source to ArticlePB_Publication
Scopus ID2-s2.0-85113300231
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Citation statistics
Document TypeJournal article
CollectionINSTITUTE OF APPLIED PHYSICS AND MATERIALS ENGINEERING
Corresponding AuthorWang, S.P.; Ng, K.W.
Affiliation1.Joint Key Laboratory of the Ministry of Education, Institute of Applied Physics and Materials Engineering, University of Macau, Avenida da Universidade, Taipa, 999078, Macao
2.Institute of Semiconductor Science and Technology, South China Normal University, Guangzhou, 510631, China
3.SCNU Qingyuan Institute of Science and Technology Innovation Co. Ltd., Qingyuan, 511517, China
First Author AffilicationINSTITUTE OF APPLIED PHYSICS AND MATERIALS ENGINEERING
Corresponding Author AffilicationINSTITUTE OF APPLIED PHYSICS AND MATERIALS ENGINEERING
Recommended Citation
GB/T 7714
Yan, S.S.,Wang, K.Y.,Xing, G.C.,et al. Robust Ultralong Lead Halide Perovskite Microwire Lasers[J]. ACS Applied Material Interfaces, 2021, 13(32), 38458-38466.
APA Yan, S.S.., Wang, K.Y.., Xing, G.C.., Xu, J.C.., Su, S.C.., Tang, Z.K.., Wang, S.P.., & Ng, K.W. (2021). Robust Ultralong Lead Halide Perovskite Microwire Lasers. ACS Applied Material Interfaces, 13(32), 38458-38466.
MLA Yan, S.S.,et al."Robust Ultralong Lead Halide Perovskite Microwire Lasers".ACS Applied Material Interfaces 13.32(2021):38458-38466.
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